Antiferromagnetic structure of FePt3 films studied by neutron scattering

Abstract

The magnetism of antiferromagnetic FexPt1-x thin films (x = 0.27 and 0.30) epitaxially grown onto MgO (110) and a-axis sapphire (alpha -Al2O3) substrates has been studied by elastic neutron and x-ray scattering. Bulk chemically ordered FePt3 exhibits an antiferromagnetic spin structure with a wave vector Q(1) =2 pi /a(1/2 1/2 0) below T(N1)similar to 160 K. For slightly Fe-rich alloys (x greater than or similar to0.26) a spin-reorientation transition ti, a second antiferromagnetic phase with a wave vector Q(2) = 2 pi /a(1/2 00) occurs below T(N2)similar to 100 K at the expense of Q(1). For increased Fe content (x similar to0.30) the Q(1) phase is strongly suppressed with a dominant Q(2) phase. For (111)-oriented films grown on a-axis sapphire the spin structure is the same as that found in the bulk. The a = 0.27 film exhibits transitions at T-N1 and T-N2. The film with x = 0.30 exhibits an almost completely suppressed Q(1) phase and a dominant Q(2) phase with an enhanced ordering temperature of T(N2)similar to 140 K. In contrast FePt3 (110) films grown onto MgO (110) exhibit only the el phase for both compositions x = 0.27 and x = 0.30 with the onset of the Q(2) phase suppressed. The distinct behavior of the films grown onto MgO from those grown onto a-axis sapphire and bulk FePt3 may be explained by higher strain and defect densities incorporated in the films grown onto MgO.

Description
Keywords
EXCHANGE BIASED FILMS, ANISOTROPY, Materials Science, Multidisciplinary, Physics, Applied, Physics, Condensed Matter, Materials Science, Physics
Citation
Maat, S., et al. (2001): Antiferromagnetic Structure of FePt₃ Films Studied by Neutron Scattering. Physical Review B, 63(13). DOI: https://doi.org/10.1103/PhysRevB.63.134426